Oxide coatings with immobilized Ce-ZSM5 as visible light photocatalysts: Scientific paper

Nikola Božović; Kristina Mojsilović; Srna Stojanović; Ljiljana Damjanović-Vasilić; Maria Serdechnova; Carsten Blawert; Mikhail L. Zheludkevich; Stevan Stojadinović; Rastko Vasilić

doi:10.2298/JSC211203058B

PDF (3.398 kB) Supplementary Material (3.66 MB)

Published: Aug 26, 2022

Updated: 26.08.2022

DOI: https://doi.org/10.2298/JSC211203058B

Keywords:

plasma electrolytic oxidation zeolites multifunctional coatings

Nikola Božović

University of Belgrade, Faculty of Physics, Studentski trg 12-16, 11000 Belgrade, Serbia: and Directorate of Measures and Precious Metals, Mike Alasa 14, 11000 Belgrade, Serbia

Kristina Mojsilović

University of Belgrade, Faculty of Physics, Studentski trg 12-16, 11000 Belgrade, Serbia

https://orcid.org/0000-0003-1424-3225

Srna Stojanović

University of Belgrade, Faculty of Physical Chemistry, Studentski trg 12-16, 11000 Belgrade, Serbia

https://orcid.org/0000-0001-9950-8303

Ljiljana Damjanović-Vasilić

University of Belgrade, Faculty of Physical Chemistry, Studentski trg 12-16, 11000 Belgrade, Serbia

Maria Serdechnova

Institute of Surface Science, Helmholtz-Zentrum Hereon, Max-Planck-Straβe 1, 21502 Geesthacht, Germany

https://orcid.org/0000-0003-1879-5510

Carsten Blawert

Institute of Surface Science, Helmholtz-Zentrum Hereon, Max-Planck-Straβe 1, 21502 Geesthacht, Germany

Mikhail L. Zheludkevich

Institute of Surface Science, Helmholtz-Zentrum Hereon, Max-Planck-Straβe 1, 21502 Geesthacht, Germany and Institute of Materials Science, Faculty of Engineering, Kiel University, Kaiserstraße 2, 24143 Kiel, Germany

Stevan Stojadinović

University of Belgrade, Faculty of Physics, Studentski trg 12-16, 11000 Belgrade, Serbia

https://orcid.org/0000-0002-6589-6296

Rastko Vasilić

Faculty of Physics, University of Belgrade, Studentski trg 12-16, 11000 Belgrade, Serbia

https://orcid.org/0000-0003-2476-7516

Abstract

The preparation and properties of oxide coatings with immobilized ZSM-5 zeolite obtained by plasma electrolytic oxidation on aluminum support were investigated and discussed. Pure and Ce-exchanged ZSM-5 were immobilized on aluminum supports from a silicate-based electrolyte under ultra-low duty cycle pulsed direct current conditions. The obtained composite coatings were characterized with respect to their morphology, phase and chemical composition, as well as photocatalytic activity and anti-corrosion properties. All mentioned properties of the obtained coatings were dependent on the processing time. The coatings with Ce-exchanged ZSM-5 showed higher photocatalytic activity and more effective corrosion protection than those with pure ZSM-5. The highest photocatalytic activity was observed for coatings processed for 30 min. It is suggested that the surface morphology, Ce-content and number of defects influenced the photocatalytic activity of the composite coatings.

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How to Cite

[1]

N. Božović, “Oxide coatings with immobilized Ce-ZSM5 as visible light photocatalysts: Scientific paper”, J. Serb. Chem. Soc., vol. 87, no. 9, pp. 1035–1048, Aug. 2022.

Issue

Vol. 87 No. 9 (2022)

Section

Physical Chemistry

This work is licensed under a Creative Commons Attribution-NonCommercial-NoDerivatives 4.0 International License.

Authors retain copyright and grant the journal right of first publication with the work simultaneously licensed under a Creative Commons Attribution license 4.0 that allows others to share the work with an acknowledgement of the work's authorship and initial publication in this journal.

Funding data

Ministarstvo Prosvete, Nauke i Tehnološkog Razvoja
Grant numbers 451-03-68/2022-14/200162;451-03-68/2022-14/200146
H2020 Marie Skłodowska-Curie Actions
Grant numbers 823942 (FUNCOAT)

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Oxide coatings with immobilized Ce-ZSM5 as visible light photocatalysts Scientific paper