Degradation of Reactive Red 120 dye by a heterogeneous sono-Fenton process with goethite deposited onto silica and calcite sand

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Published: Feb 13, 2020
DOI: https://doi.org/10.2298/JSC190506096G
Keywords:
AOPs goethite immobilization ultrasound irradiation azo dye

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Soraya Garófalo-Villalta
Departamento de Ciencias Nucleares, Facultad de Ingeniería Química y Agroindustria, Escuela Politécnica Nacional, Ladrón de Guevara E11-253, 170525 Quito
https://orcid.org/0000-0003-4181-7511
Tanya Medina-Espinosa
Departamento de Ciencias Nucleares, Facultad de Ingeniería Química y Agroindustria, Escuela Politécnica Nacion
https://orcid.org/0000-0003-4401-4618
Christian Sandoval-Pauker
Departamento de Ciencias Nucleares, Facultad de Ingeniería Química y Agroindustria, Escuela Politécnica Nacion
https://orcid.org/0000-0002-7831-331X
William Villacis
Departamento de Ciencias Nucleares, Facultad de Ingeniería Química y Agroindustria, Escuela Politécnica Nacion
https://orcid.org/0000-0001-8653-7586
Valerian Ciobotă
Rigaku Analytical Devices, Inc. 30 Upton Drive, Suite 2, Wilmington, MA 01887
https://orcid.org/0000-0003-1603-0434
Florinella Muñoz Bisesti
Departamento de Ciencias Nucleares, Facultad de Ingeniería Química y Agroindustria, Escuela Politécnica Nacion
https://orcid.org/0000-0002-5015-6455
Paul Vargas Jentzsch
Departamento de Ciencias Nucleares, Facultad de Ingeniería Química y Agroindustria, Escuela Politécnica Nacion
http://orcid.org/0000-0002-2983-5824

Abstract

The degradation of Reactive Red 120 dye (RR-120) in synthetic waters was studied. Two processes were considered: homogeneous sono-Fen­ton with iron(II) sulfate and heterogeneous sono-Fenton with synthetic goethite and goethite deposited onto silica and calcite sand (modified catalysts GS and GC, respectively). In 60 min of reaction, the homogeneous sono-Fenton pro­cess allowed a degra­dation of 98.10 %, in contrast with 96.07 % for the heterogeneous sono-Fenton process with goethite at pH 3.0. The removal of RR-120 increased when the modified catalysts were used instead of bare goe­thite. Chemical oxygen demand (COD) and total organic carbon (TOC) mea­surements showed that the highest TOC and COD removals were achieved with the homogeneous sono-Fenton process. Biochemical oxygen demand (BOD5) measurements allowed confirmed that the highest value of BOD5/COD was achieved with a heterogeneous sono-Fenton process (0.88±0.04 with the modi­fied catalyst GC), demonstrating that the biodegradability of the residual org­anic compounds was remarkably improved.

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How to Cite
[1]
S. Garófalo-Villalta, “Degradation of Reactive Red 120 dye by a heterogeneous sono-Fenton process with goethite deposited onto silica and calcite sand”, J. Serb. Chem. Soc., vol. 85, no. 1, pp. 125–140, Feb. 2020.
Issue
Vol. 85 No. 1 (2020)
Section
Environmental Chemistry

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